Figure 6.1: r ≈ 2.5 nmcorral grid spectrum. Top left: effective dI/dV map from grid at ∼ 7 mV (marked by vertical line, top right). Top right: six of the 10,000 dI/dV spectra comprising the grid on the left. The shade of the spectra (right) correspond to the location with a dot of the same color (left). For example, on top of the Co (blue and orange, left) corresponds to the most prominent Fano lineshape (blue and orange, right), whereas the spectrum ∼ 1.5 nm from the Co (pink, left) does not show a prominent Fano resonance.Bottom: results from fitting equation 1.6 to grid spectrum.Bottom left:
corral topography.Bottom right:spatial maps of parameters acquired from fitting spectra from within the dashed line box on the left over energy range−15 mV to20 mV, fixing ϵ0 = 8.3 mV. These results can be used to fit, for example, decay ofq as a function of distance from the Co to equation 1.7, or to improve the quality of the data represented in figure 3.10.
100 75 50 25 0 25 50 75 100
Fit initial guess (0,w,q,a,b,c) 6.94, 14.66, 0.22 68.72, -3.57, 223.08 Corral radius: 2.693 nm Distance to Co: 0.054 nm
Ag 2021-08-09 2p5 nm radius/pm 100mV line spectrum across corral Createc2_210809.154356.L0024.VERT
Figure 6.2: Top: Example output from script to extract corral radius from topography.
Bottom: Example output from script to extract parameters from Fano fit to spectral data.
39
(a)8 mVconstant height map of4.5 nmradius corral.
(b)45 mVconstant height map.
(c)125 mVconstant height map. (d)175 mVconstant height map.
Figure 6.3: Constant height dI/dV maps of 4.65 nm radius corral. Set point current 100 pA, lock-in frequency746 Hz, lock-in amplitude1 mV.
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